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Superior multiphoton absorption properties in colloidal Mn-doped CsPbCl3 two-dimensional nanoplatelets

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Abstract

We have studied the two- and three-photon absorption (2PA and 3PA) properties of Mn-doped CsPbCl3 two-dimensional nanoplatelets (2D NPs) and cubic nanocrystals. Compared with their cubic counterparts, the Mn-doped 2D NPs exhibit stronger quantum confinement effects that can more efficiently enhance their dopant-carrier exchange interactions and multiphoton absorption. More specifically, the maximum volume-normalized 2PA and 3PA cross sections of the 2D NPs were 6.8 and 7.2 times greater than those of their cubic counterparts, respectively, reaching up to 1237 GM/nm3 in the visible light band and 2.24×10?78 cm6·s2·photon?2/nm3 in the second biological window, respectively.

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DOI:10.1364/prj.6.001021

所属栏目:Nonlinear optics

基金项目:Shenzhen Basic Research Project of Science and Technology (JCYJ20150324141711581, JCYJ20170302142433007); Postgraduate Innovation Development Fund Project of Shenzhen University (PIDFP-ZR2018007).

收稿日期:2018-07-12

录用日期:2018-09-05

网络出版日期:2018-09-05

作者单位    点击查看

Tingchao He:College of Physics and Energy, Shenzhen University, Shenzhen 518060, China
Junzi Li:College of Physics and Energy, Shenzhen University, Shenzhen 518060, China
Xin Qiu:College of Physics and Energy, Shenzhen University, Shenzhen 518060, China
Shuyu Xiao:College of Physics and Energy, Shenzhen University, Shenzhen 518060, China
Xiaodong Lin:College of Physics and Energy, Shenzhen University, Shenzhen 518060, China

联系人作者:Xiaodong Lin(linxd@szu.edu.cn)

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引用该论文

Tingchao He, Junzi Li, Xin Qiu, Shuyu Xiao, and Xiaodong Lin, "Superior multiphoton absorption properties in colloidal Mn-doped CsPbCl3 two-dimensional nanoplatelets," Photonics Research 6(11), 1021-1027 (2018)

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