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量子级联激光光谱在土壤生态系统中的应用 (封面文章)

Application of Quantum-Cascade Laser Spectroscopy to Soil Ecosystems (Cover Paper)

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Soil respiration is the main process of carbon and nitrogen circulation between the earth and atmosphere. Real-time in-situ measurement of gas emissions from different ecological soil environments is a powerful tool for studying the dynamic processes of atmospheric-greenhouse-gas formation, transfer, and consumption, which provides the key scientific basis for revealing the main processes of carbon and nitrogen ecosystem cycling and environmental evolution. In this paper, we describe the development of a laser-spectroscopy system based on a room-temperature, continuous-wave, quantum-cascade laser (RT-CW-QCL), a long-path optical-absorption cell, and a direct-absorption spectroscopic detection technology for the high-sensitivity and high-precision analysis of CO and N2O gas-exchange processes between soil samples under different ecological environments and ambient air. The results show that soil samples from four different ecological environments (i.e., reed, pond, organic, and grassland soils) exhibit visibly different CO and N2O release and absorption processes.









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刘宁武:安徽大学物理与材料科学学院, 安徽 合肥 230601
许林广:安徽大学物理与材料科学学院, 安徽 合肥 230601
周胜:安徽大学物理与材料科学学院, 安徽 合肥 230601
何天博:安徽大学物理与材料科学学院, 安徽 合肥 230601
李劲松:安徽大学物理与材料科学学院, 安徽 合肥 230601



【1】Zhang Y S, Ding H, Qin S J. Progress in the studies of nitrogen denitrification and N2O emission in agro-ecosystem [J]. Chinese Agricultural Science Bulletin. 2010, 26(6): 253-259.
张玉树, 丁洪, 秦胜金. 农业生态系统中氮素反硝化作用与N2O排放研究进展 [J]. 中国农学通报. 2010, 26(6): 253-259.

【2】Yuan W H, Zhang Y J, Wang J G, et al. Study on the extreme cold and warm weather climate events in Shandong Province in recent 45 years by using the detection method based on median [J]. Meteorological and Environmental Research. 2010, 1(11): 42-55.

【3】Griggs D J, Noguer M. Climate change 2001: the scientific basis. Contribution of working group I to the third assessment report of the intergovernmental panel on climate change [J]. Weather. 2002, 57(8): 267-269.

【4】Frankenberg C, Bergamaschi P, Butz A, et al. Tropical methane emissions: a revised view from SCIAMACHY onboard ENVISAT [J]. Geophysical Research Letters. 2008, 35(15): L15811.

【5】King G M, Weber C F. Distribution, diversity and ecology of aerobic CO-oxidizing bacteria [J]. Nature Reviews Microbiology. 2007, 5(2): 107-118.

【6】Wu R J, Wu J G, Tsai T K, et al. Use of cobalt oxide CoOOH in a carbon monoxide sensor operating at low temperatures [J]. Sensors and Actuators B: Chemical. 2006, 120(1): 104-109.

【7】Shemshad J, Aminossadati S M, Actuators B: Chemical. 2012, 171/172: 77-92.

【8】Wang Q, Chang J, Wei W, et al. Dual-beam wavelength modulation spectroscopy for sensitive detection of water vapor [J]. Applied Physics B. 2014, 117(4): 1015-1023.

【9】Gao Q, Zhang Y G, Yu J, et al. Tunable multi-mode diode laser absorption spectroscopy for methane detection [J]. Sensors and Actuators A: Physical. 2013, 199: 106-110.

【10】Kan R F, Liu W Q, Zhang Y J, et al. Tunable diode laser absorption spectrometer monitors the ambient methane with high sensitivity [J]. Chinese Journal of Lasers. 2005, 32(9): 1217-1220.
阚瑞峰, 刘文清, 张玉钧, 等. 可调谐二极管激光吸收光谱法监测环境空气中甲烷的浓度变化 [J]. 中国激光. 2005, 32(9): 1217-1220.

【11】Li J S, Deng H, Sun J, et al. Simultaneous atmospheric CO, N2O and H2O detection using a single quantum cascade laser sensor based on dual-spectroscopy techniques [J]. Sensors and Actuators B: Chemical. 2016, 231: 723-732.

【12】Cui X J, Dong F Z, Chen W D, et al. Nitrous acid measurement based on room-temperature continuous wave quantum cascade laser [J]. Acta Optica Sinica. 2013, 33(4): 0430002.
崔小娟, 董凤忠, 陈卫东, 等. 基于室温连续量子级联激光器的HONO气体检测 [J]. 光学学报. 2013, 33(4): 0430002.

【13】Ma Y F, Lewicki R, Razeghi M, et al. QEPAS based ppb-level detection of CO and N2O using a high power CW DFB-QCL [J]. Optics Express. 2013, 21(1): 1008-1019.

【14】Tong Y, Ma Y F. Research progress of the trace gas sensing based on quartz-enhanced photoacoustic spectroscopy [J]. Journal of Liaocheng University(Nat. Sci.). 2019, 32(2): 34-41.
佟瑶, 马欲飞. 基于石英增强光声光谱的痕量气体传感技术研究进展 [J]. 聊城大学学报(自然科学版). 2019, 32(2): 34-41.

【15】Wei M, Liu J G, Kan R F, et al. Study on detection of greenhouse gases based on quantum cascade laser [J]. Acta Optica Sinica. 2014, 34(12): 1230003.
魏敏, 刘建国, 阚瑞峰, 等. 基于量子级联激光器的温室气体测量方法研究 [J]. 光学学报. 2014, 34(12): 1230003.

【16】Wei W, Chang J, Huang Q J, et al. Wavelength modulation spectroscopy with signal-reference beam method for highly sensitive gas detection [J]. Applied Physics B. 2015, 118(1): 75-83.

【17】Zhou C, Zhang L, Li J S. Detection of atmospheric multi-component based on a single quantum cascade laser [J]. Acta Physica Sinica. 2017, 66(9): 094203.
周超, 张磊, 李劲松. 基于单个量子级联激光器的大气多组分测量方法 [J]. 物理学报. 2017, 66(9): 094203.

【18】Bruhn D, Albert K R, Mikkelsen T N, et al. UV-induced carbon monoxide emission from living vegetation [J]. Biogeosciences. 2013, 10(12): 7877-7882.

【19】van Asperen H, Warneke T, Sabbatini S, et al. . The role of photo- and thermal degradation for CO2 and CO fluxes in an arid ecosystem [J]. Biogeosciences. 2015, 12(13): 4161-4174.

【20】Pihlatie M, Rannik ü, Haapanala S, et al. Seasonal and diurnal variation in CO fluxes from an agricultural bioenergy crop [J]. Biogeosciences. 2016, 13(19): 5471-5485.

【21】Sun W. Kooijmans L M J, Maseyk K, et al. Soil fluxes of carbonyl sulfide (COS), carbon monoxide, and carbon dioxide in a boreal forest in southern Finland [J]. Atmospheric Chemistry and Physics. 2018, 18(2): 1363-1378.

【22】Singh B P, Hatton B J, Singh B, et al. Influence of biochars on nitrous oxide emission and nitrogen leaching from two contrasting soils [J]. Journal of Environment Quality. 2010, 39(4): 1224-1235.

【23】Cui F, Yan G X, Zhou Z X, et al. Annual emissions of nitrous oxide and nitric oxide from a wheat-maize cropping system on a silt loam calcareous soil in the North China Plain [J]. Soil Biology and Biochemistry. 2012, 48: 10-19.

【24】Sakata R, Shimada S, Arai H, et al. Effect of soil types and nitrogen fertilizer on nitrous oxide and carbon dioxide emissions in oil palm plantations [J]. Soil Science and Plant Nutrition. 2015, 61(1): 48-60.

【25】Ruan L L, Robertson G P. Reduced snow cover increases wintertime nitrous oxide (N2O) emissions from an agricultural soil in the upper US midwest [J]. Ecosystems. 2017, 20(5): 917-927.


Liu Ningwu,Xu Linguang,Zhou Sheng,He Tianbo,Li Jingsong. Application of Quantum-Cascade Laser Spectroscopy to Soil Ecosystems[J]. Acta Optica Sinica, 2019, 39(11): 1130001

刘宁武,许林广,周胜,何天博,李劲松. 量子级联激光光谱在土壤生态系统中的应用[J]. 光学学报, 2019, 39(11): 1130001

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