首页 > 论文 > 中国激光 > 47卷 > 9期(pp:913001--1)

TiN纳米粒子增强CdSe/Al2O3异质结荧光的研究

Enhanced Fluorescence of CdSe/Al2O3 Heterojunctions Enabled by TiN Nanoparticles

  • 摘要
  • 论文信息
  • 参考文献
  • 被引情况
  • PDF全文
分享:

摘要

利用TiN纳米粒子对CdSe量子点和多孔Al2O3薄膜构成的异质结的表面荧光增强效应进行了实验研究。采用电化学沉积的方法,将TiN纳米粒子沉积于多孔Al2O3薄膜表面,再将胶体CdSe量子点自组装于TiN/Al2O3薄膜的表面,进而制备了CdSe/TiN/Al2O3异质结。同时,利用扫描近场光学显微镜测量了CdSe/TiN/Al2O3异质结的表面增强荧光效应。结果表明,由于TiN具有良好的电子传输特性,提高了CdSe量子点和多孔Al2O3薄膜之间的光生电子转移效率,进而增强了多孔Al2O3薄膜界面的荧光。该研究结果可广泛应用于光伏、光显示、光传感及纳米生物成像等领域。

Abstract

The enhanced fluorescence effect of the heterojunction of CdSe quantum dots and a porous Al2O3 film was experimentally studied by using TiN nanoparticles (NPs). TiN NPs were deposited on the surface of porous Al2O3 film. Then, the CdSe QDs were self-assembled on the surface of TiN/Al2O3 film to prepare the CdSe/TiN/Al2O3 heterojunction. At the same time, the surface enhanced fluorescence effect was observed on the platform of a scanning near-field optical microscope. The results have showed that the interfacial fluorescence from the porous Al2O3 film was enhanced due to the increase of poto-generated carriers resulted in by TiN Nps from the CdSe QDs to the porous Al2O3 film. These results based on this paper could be widely applied for many fields of photovoltaic, lightshows, optical sensors devices and nano-biological imaging system.

广告组1 - 空间光调制器+DMD
补充资料

中图分类号:O432

DOI:10.3788/CJL202047.0913001

所属栏目:微纳光学

基金项目:国家自然科学基金、贵州省科技支撑项目、中央引导地方科技发展专项、贵州省人才团队项目;

收稿日期:2020-03-16

修改稿日期:2020-04-13

网络出版日期:2020-09-01

作者单位    点击查看

刘鹏程:贵州大学贵州省光电子技术及应用重点实验室, 贵州 贵阳 550025
昌梦雨:贵州大学贵州省光电子技术及应用重点实验室, 贵州 贵阳 550025贵州大学医学院, 贵州 贵阳 550025
白忠臣:贵州大学贵州省光电子技术及应用重点实验室, 贵州 贵阳 550025贵州大学医学院, 贵州 贵阳 550025
秦水介:贵州大学贵州省光电子技术及应用重点实验室, 贵州 贵阳 550025

联系人作者:秦水介(shuijie_qin@sina.com)

备注:国家自然科学基金、贵州省科技支撑项目、中央引导地方科技发展专项、贵州省人才团队项目;

【1】Bai Z C, Hao L C, Zhang Z P, et al. Enhanced photoluminescence of corrugated Al2O3 film assisted by colloidal CdSe quantum dots [J]. Nanotechnology. 2017, 28(20): 205206.

【2】Fort E, Grésillon S. Surface enhanced fluorescence [J]. Journal of Physics D Applied Physics. 2008, 41(1): 13001.

【3】Li J L, Gu M. Surface plasmonic gold nanorods for enhanced two-photon microscopic imaging and apoptosis induction of cancer cells [J]. Biomaterials. 2010, 31(36): 9492-9498.

【4】Borisov S M, Wolfbeis O S. Optical biosensors [J]. Chemical Reviews. 2008, 108(2): 423-461.

【5】Rizzo R, Alvaro M, Danz N, et al. Bloch surface wave enhanced biosensor for the direct detection of Angiopoietin-2 tumor biomarker in human plasma [J]. Biomedical Optics Express. 2018, 9(2): 529.

【6】Zhang W X, Zhang X R, Qin C B, et al. Continuous laser induced photoluminescence enhancement of Au nanorods [J]. Laser & Optoelectronics Progress. 2019, 56(20): 202410.
张文学, 张晓荣, 秦成兵, 等. 连续激光诱导金纳米棒荧光增强效应 [J]. 激光与光电子学进展. 2019, 56(20): 202410.

【7】Yang J, Lee J, Lee J Y, et al. Photocurrent enhancement of CdSe quantum-dot sensitized solar cells incorporating single-walled carbon nanotubes [J]. Journal of Nanoscience and Nanotechnology. 2018, 18(2): 1347-1350.

【8】Yang J, Park T, Lee J, et al. Performance enhancement of 3-mercaptopropionic acid-capped CdSe quantum-dot sensitized solar cells incorporating single-walled carbon nanotubes [J]. Journal of Nanoscience and Nanotechnology. 2016, 16(3): 2710-2714.

【9】Gracie K, Moores M, Smith W E, et al. Preferential attachment of specific fluorescent dyes and dyelabeled DNA sequences in a surface enhanced Raman scattering multiplex [J]. Analytical Chemistry. 2016, 88(2): 1147-1153.

【10】Peng M, Bai Z C, Li X J, et al. Controlling wide-spectrum fluorescence on Au/ZnSe multi-heterojunction [J]. Applied Physics A. 2018, 124(7): 1-6.

【11】Bai Z C, Hao L C, Huang Z L, et al. Enhancement effect of defect fluorescence of ZnSe quantum dots on a heterojuction of ZnSe quantum dots and gold nanoparticles [J]. Methods and Applications in Fluorescence. 2017, 5(4): 045001.

【12】Cheng C, Mao M. Photo-stability and time-resolved photoluminescence study of colloidal CdSe/ZnS quantum dots passivated inAl2O3 using atomic layer deposition [J]. Journal of Applied Physics. 2016, 120(8): 083103.

【13】Zhang Y, Bai Z C, Huang Z L, et al. Influence of distance between CdSe quantum dot and gold nanoparticle on system fluorescence [J]. Laser & Optoelectronics Progress. 2018, 55(7): 072601.
张莹, 白忠臣, 黄兆岭, 等. 金纳米粒子与CdSe量子点间的距离对体系荧光的影响 [J]. 激光与光电子学进展. 2018, 55(7): 072601.

【14】Dixit S K, Bhatnagar C, Kumari A, et al. Development and characterization of PCDTBT: , 2014.

【15】Dayneko S, Tameev A, Tedoradze M, et al. Hybrid bulk heterojunction solar cells based on low band gap polymers and CdSe nanocrystals [J]. Proceedings of SPIE. 2014, 8981: 898113.

【16】Patel M, Sahu S, Verma A K, et al. Solution processed solar cells based onin situ synthesis of CdSe quantum dots[C]∥2017 International Conference on Energy. 1-2 Aug. 2017, Chennai, India. New York: , 2017, 1683-1687.

【17】Laatar F, Moussa H, Alem H, et al. CdSe nanorod/TiO2 nanoparticle heterojunctions with enhanced solar- and visible-light photocatalytic activity [J]. Beilstein Journal of Nanotechnology. 2017, 8: 2741-2752.

【18】Chen W W, Yu S, Zhong Y Q, et al. Effect of electron transfer on the photocatalytic hydrogen evolution efficiency of faceted TiO2/CdSe QDs under visible light [J]. New Journal of Chemistry. 2018, 42(7): 4811-4817.

【19】Kozlova E A, Kurenkova A Y, Semeykina V S, et al. Effect oftitania regular macroporosity on the photocatalytic hydrogen evolution on Cd1-xZnxS/TiO2 catalysts under visible light [J]. ChemCatChem. 2015, 7(24): 4108-4117.

【20】Chatterjee S. Indian Institute of Engineering Science and Technology India, Sarkar J, et al. Effect of anodizing medium on the morphology and photoluminescent property of porous alumina film [J]. GSTF Journal of Engineering Technology. 2017, 4(2): 59-62.

【21】Ismail A K, Ibrahim N H, Shamsuddin K A, et al. A practical approach in porous medium combustion for domestic application:a review [J]. IOP Conference Series: Materials Science and Engineering. 2018, 370: 012004.

【22】Kim Y M. RheeG H, Ko C H, et al. Catalytic pyrolysis of Korean pine (pinus koraiensis) nut shell over mesoporous Al2O3 [J]. Journal of Nanoscience and Nanotechnology. 2018, 18(2): 1351-1355.

【23】Guarnera S. AbateA, Zhang W, et al. Improving the long-term stability of perovskite solar cells with a porous Al2O3 buffer-layer [J]. Journal of Physical Chemistry Letters. 2015, 6(3): 432-437.

【24】Zhang J, Yue D, Xia T F, et al. A luminescent metal-organic framework film fabricated on porous Al2O3 substrate for sensitive detecting ammonia [J]. Microporous and Mesoporous Materials. 2017, 253: 146-150.

【25】Guo H S, Li W F. Effects of Al2O3 crystal types on morphologies, formation mechanisms of mullite and properties of porous mullite ceramics based on kyanite [J]. Journal of the European Ceramic Society. 2018, 38(2): 679-686.

【26】Rose V. 105(7): 07C902 [J]. Franchy R. The band gap of ultrathin amorphous, well-ordered Al2O3 films on CoAl, 100, measured by scanning tunneling spectroscopy. Journal of Applied Physics. 2009.

【27】Bai Z C, Huang Z L, Hao L C, et al. Identifying defects in thin film of high power laser lens by using near field microimaging method [J]. Chinese Journal of Lasers. 2017, 44(1): 0103001.
白忠臣, 黄兆岭, 郝礼才, 等. 近场显微成像法识别高功率激光镜片薄膜内部缺陷 [J]. 中国激光. 2017, 44(1): 0103001.

【28】Bai Z C, Peng M, Zhang Z P, et al. Enhanced and broadened fluorescence of ZnSe quantum dots enabled by the fluorescence energy transfer system of ZnSe quantum dots and gold nanoparticles [J]. Applied Optics. 2018, 57(28): 8437-8442.

【29】Murai S, Fujita K, Daido Y, et al. Plasmonic arrays of titanium nitride nanoparticles fabricated from epitaxial thin films [J]. Optics Express. 2016, 24(2): 1143-1153.

【30】Naik G V, Schroeder J, Ni XJ, et al. Titanium nitride as a plasmonic material for visible and near-infrared wavelengths [J]. Optical Materials Express. 2012, 3(10): 1658-1659.

【31】Zgrabik C M, Hu E L. Optimization of sputtered titanium nitride as a tunable metal for plasmonic applications [J]. Optical Materials Express. 2015, 5(12): 2786-2797.

【32】Jaramillo-Quintero O A, Triana M A, Rincon M E. Optimization of charge transfer and transport processes at the CdSe quantum dots/TiO2 nanorod interface by TiO2 interlayer passivation [J]. Journal of Physics D: Applied Physics. 2017, 50(23): 235305.

【33】Naldoni A, Guler U, Wang Z X, et al. Broadband hot-electron collection for solar water splitting with plasmonic titanium nitride [J]. Advanced Optical Materials. 2017, 5(15): 1601031.

【34】Zhao Y, Song Z M, Jin J B, et al. Electrochemical corrosion properties of Ti-5%TiN composites formed by selective laser melting in hank''''s solution [J]. Chinese Journal of Lasers. 2019, 46(9): 0902005.
赵宇, 宋振明, 金剑波, 等. 激光选区熔化成形Ti-5%TiN复合材料在Hank溶液中的电化学腐蚀性能 [J]. 中国激光. 2019, 46(9): 0902005.

【35】Avasarala B, Haldar P. Durability and degradation mechanism of titanium nitride based electrocatalysts for PEM (proton exchange membrane) fuel cell applications [J]. Energy. 2013, 57: 545-553.

【36】Gao L, Gst?ttner J, Emling R, et al. Thermal stability of titanium nitride diffusion barrier films for advanced silver interconnects [J]. Microelectronic Engineering. 2004, 76(1/2/3/4): 76-81.

【37】Endres R, Krauss T, Wessely F, et al. Damascene metal gate technology for damage-free gate-last high-k process integration[C]∥2009 3rd International Conference on Signals. 6-8 Nov. 2009, Medenine, Tunisia. New York: , 2009, 1-3.

【38】Hao L, Bai Z, Qin S, et al. The effect of differential temperatures on the latent heat in the nucleation of CdSe quantum dots [J]. Journal of Semiconductors. 2017, 38(4): 042004.

【39】Bai Z C, Hao L C, Zhang Z P, et al. Measuring photoluminescence spectra of self-assembly array nanowire of colloidal CdSe quantum dots using scanning near-field optics microscopy [J]. Functional Materials Letters. 2016, 09(3): 1650040.

【40】Guo Y, He X, Liu X, et al. One-step implementation of plasmon enhancement and solvent annealing effects for air-processed high-efficiency perovskite solar cells [J]. Journal of Materials Chemistry. 2018, 6(47): 24036-24044.

引用该论文

Liu Pengcheng,Chang Mengyu,Bai Zhongchen,Qin Shuijie. Enhanced Fluorescence of CdSe/Al2O3 Heterojunctions Enabled by TiN Nanoparticles[J]. Chinese Journal of Lasers, 2020, 47(9): 0913001

刘鹏程,昌梦雨,白忠臣,秦水介. TiN纳米粒子增强CdSe/Al2O3异质结荧光的研究[J]. 中国激光, 2020, 47(9): 0913001

您的浏览器不支持PDF插件,请使用最新的(Chrome/Fire Fox等)浏览器.或者您还可以点击此处下载该论文PDF