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Two-photon absorption towards pulse modulation in mechanically exfoliated and CVD monolayer cascaded MoS2 structures

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Abstract

Mechanical exfoliation (ME) and chemical vapor deposition (CVD) MoS2 monolayers have been extensively studied, but the large differences of nonlinear optical performance between them have never been clarified. Here, we prepared MoS2 monolayers using ME and CVD methods and investigated the two-photon absorption (TPA) response and its saturation. We found that the TPA coefficient of the ME monolayer was about (1.88 ± 0.21) × 103 cm/GW, nearly two times that of the CVD one at (1.04 ± 0.15) × 103 cm/GW. Furthermore, we simulated and compared the TPA-induced optical pulse modulation in multilayer cascaded structures, which is instructive and meaningful for the design of optical devices such as a beam shaper and optical limiter.

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DOI:10.3788/COL201917.081901

所属栏目:Nonlinear optics

基金项目:This work was supported by the National Natural Science Foundation of China (NSFC) (Nos. 61675217 and 11874370), the Strategic Priority Research Program of CAS (No. XDB16030700), the Key Research Program of Frontier Science of CAS (No. QYZDB-SSW-JSC041), the Program of Shanghai Academic Research Leader (No. 17XD1403900), the Natural Science Foundation of Shanghai (No. 18ZR1444700), the Shanghai Rising-Star Program (A Type 19QA1410000), and the Youth Innovation Promotion Association, CAS.

收稿日期:2019-03-13

录用日期:2019-04-25

网络出版日期:2019-07-17

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Yafeng Xie:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, ChinaCenter of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
Saifeng Zhang:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Xiaoyan Zhang:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Ningning Dong:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Ivan M. Kislyakov:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Song Luo:State Key Laboratory of Surface Physics, Key Laboratory of Micro and Nano Photonic Structures of Ministry of Education, Department of Physics, Collaborative Innovation Center of Advanced Microstructures, Fudan University, Shanghai 200433, China
Zhanghai Chen:State Key Laboratory of Surface Physics, Key Laboratory of Micro and Nano Photonic Structures of Ministry of Education, Department of Physics, Collaborative Innovation Center of Advanced Microstructures, Fudan University, Shanghai 200433, China
Jean-Michel Nunzi:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, ChinaDepartment of Physics, Engineering Physics & Astronomy and Department of Chemistry, Queen’s University, Kingston K7L-3N6, Ontario, Canada
Long Zhang:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Jun Wang:Laboratory of Micro-Nano Photonic and Optoelectronic Materials and Devices, Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China

联系人作者:Saifeng Zhang(sfzhang@siom.ac.cn); Jun Wang( jwang@siom.ac.cn);

备注:This work was supported by the National Natural Science Foundation of China (NSFC) (Nos. 61675217 and 11874370), the Strategic Priority Research Program of CAS (No. XDB16030700), the Key Research Program of Frontier Science of CAS (No. QYZDB-SSW-JSC041), the Program of Shanghai Academic Research Leader (No. 17XD1403900), the Natural Science Foundation of Shanghai (No. 18ZR1444700), the Shanghai Rising-Star Program (A Type 19QA1410000), and the Youth Innovation Promotion Association, CAS.

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引用该论文

Yafeng Xie, Saifeng Zhang, Xiaoyan Zhang, Ningning Dong, Ivan M. Kislyakov, Song Luo, Zhanghai Chen, Jean-Michel Nunzi, Long Zhang, Jun Wang, "Two-photon absorption towards pulse modulation in mechanically exfoliated and CVD monolayer cascaded MoS2 structures," Chinese Optics Letters 17(8), 081901 (2019)

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