量子电子学报, 2018, 35 (1): 54, 网络出版: 2018-01-30   

H+2分子谐波发射的空间分布

Spatial distribution of molecular harmonic emission from H+2
刘航 1,*冯立强 2,3刘辉 3
作者单位
1 辽宁工业大学化学与环境工程学院, 辽宁 锦州 121001
2 中国科学院大连化学物理研究所分子反应动力学国家重点实验室, 辽宁 大连 116023
3 辽宁工业大学理学院, 辽宁 锦州 121001
摘要
理论研究了H+2分子发射高次谐波的空间分布情况。结果表明:分子谐波主要发生在两个H核附近。当核间距离较小时, 两个H核发射谐波强度几乎一致。核间距离增大,正向H核发射谐波强度大于负向H核。随着空间非均匀激光场的引入,H+2分子在较小核间距离时, 负向H核发射谐波强度略大于正向H核;在较大核间距离时,正向H核发射谐波强度大于负向H核。 随着空间非均匀激光场引入位置从负向移动到正向(-100 a.u.到100 a.u.),正向H核发射谐波强度逐渐减小。通过叠加谐波可获得脉宽在66 as和 62 as的超短阿秒脉冲。
Abstract
The spatial distribution of high-order harmonic generation from H+2 molecules is theoretically investigated. Results show that the molecular harmonic emission mainly occurs around two H nuclei. When the internuclear distance is relatively small, the harmonic intensities of the two H nuclei are almost the same. The harmonic intensity emitted by the positive-H nucleus is higher than that of the negative-H nucleus with the internuclear distance increasing. With the introduction of the spatial inhomogeneous laser field, the harmonic intensity emitted by the negative-H nucleus is slightly higher than that of the positive-H nucleus when the internuclear distance of H+2 molecules is relatively small. The harmonic intensity emitted by the positive-H nucleus is higher than that of the negative-H nucleus when the internuclear distance is larger. As the spatial position of the space inhomogeneous laser field shifts from negative to positive(from -100 a.u. to 100 a.u.), the harmonic intensity emitted by the positive-H nucleus decreases gradually. The ultrashort attosecond pulses with durations of 66 as and 62 as can be obtained by superposition of harmonics.

刘航, 冯立强, 刘辉. H+2分子谐波发射的空间分布[J]. 量子电子学报, 2018, 35(1): 54. LIU Hang, FENG Liqiang, LIU Hui. Spatial distribution of molecular harmonic emission from H+2[J]. Chinese Journal of Quantum Electronics, 2018, 35(1): 54.

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