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Dynamical analysis of the effect of elliptically polarized laser pulses on molecular alignment and orientation

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Abstract

In this Letter, we study the molecular alignment and orientation driven by two elliptically polarized laser pulses. It is shown that the field-free molecular alignment can be achieved in a three-dimensional (3D) case, while the field-free molecular orientation is only along the x and y directions, and that the field-free alignment and orientation along different axes are related to the populations of the rotational states. It is demonstrated that changing the elliptic parameter is efficient for controlling both in-pulse and post-pulse molecular alignment and orientation. The delay time also has an influence on the field-free molecular alignment and orientation.

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DOI:10.3788/col201816.103201

所属栏目:Ultrafast optics

基金项目:This work was supported by the National Natural Science Foundation of China (No. 11674198) and the Taishan Scholar Project of Shandong Province.

收稿日期:2018-06-26

录用日期:2018-08-27

网络出版日期:2018-09-20

作者单位    点击查看

Jingsong Liu:School of Physics and Electronics, Shandong Normal University, Jinan 250358, China
Qiyuan Cheng:School of Physics and Electronics, Shandong Normal University, Jinan 250358, China
Daguang Yue:School of Physics and Electronics, Shandong Normal University, Jinan 250358, China
Xucong Zhou:School of Physics and Electronics, Shandong Normal University, Jinan 250358, China
Qingtian Meng:School of Physics and Electronics, Shandong Normal University, Jinan 250358, China

联系人作者:Qingtian Meng(qtmeng@sdnu.edu.cn)

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引用该论文

Jingsong Liu, Qiyuan Cheng, Daguang Yue, Xucong Zhou, Qingtian Meng, "Dynamical analysis of the effect of elliptically polarized laser pulses on molecular alignment and orientation," Chinese Optics Letters 16(10), 103201 (2018)

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