Photonics Research, 2020, 8 (9): 09000A31, Published Online: Sep. 3, 2020  

Mode selection and high-quality upconversion lasing from perovskite CsPb2Br5 microplates Download: 618次

Author Affiliations
1 State Key Laboratory of High Field Laser Physics and CAS Center for Excellence in Ultra-intense Laser Science, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS), Shanghai 201800, China
2 Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou 310024, China
3 School of Physical Science and Technology, ShanghaiTech University, Shanghai 200031, China
4 Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
5 Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), College of Optoelectronic Engineering, Chongqing University, Chongqing 400044, China
6 e-mail: dujuan@mail.siom.ac.cn
7 e-mail: xstang@cqu.edu.cn
8 e-mail: lengyuxinn@mail.siom.ac.cn
Abstract
In recent years, halide perovskite nanostructures have had great advances and have opened up a bright future for micro/nanolasers. However, upconversion lasing by two-photon excitation with mode selection and high quality factor in one device is still rarely reported. Herein, two lasing modes are demonstrated in the all-inorganic perovskite CsPb2Br5 microplates with subwavelength thickness and uniform square shape. The net optical gain is quickly established in less than 1 ps and persists more than 30 ps, revealed by ultrafast transient absorption spectroscopy. The temperature-dependent low-threshold amplified spontaneous emission confirms the net gain for stimulated emission with a high characteristic temperature of 403 K, far surpassing the all-inorganic CsPbBr3 semiconductor gain media. Remarkably, upconversion lasing based on two kinds of microcavity effects, Fabry–Pérot and whispering-gallery modes, from the microplates at room temperature is successfully achieved with a low threshold operating in multi- or single-mode, respectively. Surprisingly, the quality factor (3551) is among the best values obtained from perovskite micro/nanoplate upconversion lasers without an external cavity. Moreover, the highly stable chromaticity with color drift only less than 0.1 nm also outbalances the all-inorganic CsPbBr3 ones. These superior performances of CsPb2Br5 microplate lasing with a facile solution synthesis procedure will offer a feasible structure to fabricate specific functionalities for high-performance frequency upconversion micro/nanoscale photonic integrated devices.

Zhengzheng Liu, Chunwei Wang, Zhiping Hu, Juan Du, Jie Yang, Zeyu Zhang, Tongchao Shi, Weimin Liu, Xiaosheng Tang, Yuxin Leng. Mode selection and high-quality upconversion lasing from perovskite CsPb2Br5 microplates[J]. Photonics Research, 2020, 8(9): 09000A31.

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