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Broadband mid-infrared second harmonic generation using epitaxial polydomain barium titanate thin films [Editors' Pick]

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Abstract

The mid-infrared (mid-IR) second-order optical nonlinearity of the barium titanate (BTO) thin films was characterized by second harmonic generation (SHG). The epitaxial BTO thin films were grown on strontium titanate substrates by pulsed-laser deposition. From the azimuthal-dependent polarized SHG measurements, the tensorial optical nonlinear coefficients, dij, and ferroelectric domain fraction ratio, δAY/δAz, were resolved. Strong SHG signals were obtained at the pumping laser wavelength λ between 3.0 and 3.6 μm. The SHG intensity was linearly dependent upon the square of the pumping laser power. The broadband mid-IR optical nonlinearity enables BTO thin films for applications in chip-scale quantum optics and nonlinear integrated photonic circuits.

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DOI:10.1364/PRJ.7.001193

所属栏目:Optical and Photonic Materials

基金项目:Texas A&M University10.13039/100007904; National Science Foundation10.13039/100000001; Brookhaven National Laboratory10.13039/100006231;

收稿日期:2019-06-03

录用日期:2019-08-25

网络出版日期:2019-09-29

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Junchao Zhou:Department of Electrical and Computer Engineering, Texas A&M University, College Station, Texas 77843, USADepartment of Materials Science and Engineering, Texas A&M University, College Station, Texas 77843, USACenter for Remote Health Technologies and Systems, Texas A&M University, College Station, Texas 77843, USA
Wenrui Zhang:The Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton, New York 11973, USA
Mingzhao Liu:The Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton, New York 11973, USA
Pao Tai Lin:Department of Electrical and Computer Engineering, Texas A&M University, College Station, Texas 77843, USADepartment of Materials Science and Engineering, Texas A&M University, College Station, Texas 77843, USACenter for Remote Health Technologies and Systems, Texas A&M University, College Station, Texas 77843, USA

联系人作者:Pao Tai Lin(paolin@ece.tamu.edu)

备注:Texas A&M University10.13039/100007904; National Science Foundation10.13039/100000001; Brookhaven National Laboratory10.13039/100006231;

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引用该论文

Junchao Zhou, Wenrui Zhang, Mingzhao Liu, and Pao Tai Lin, "Broadband mid-infrared second harmonic generation using epitaxial polydomain barium titanate thin films," Photonics Research 7(10), 1193-1199 (2019)

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