光学学报, 2020, 40 (8): 0802001, 网络出版: 2020-04-13
波长和偏振依赖的O2分子强激光场单电离 下载: 993次
Wavelength- and Polarization-Dependent Single Ionization of O2 in Strong Laser Fields
原子与分子物理学 单电离 O2分子 强激光场 波长和偏振依赖 atomic and molecular physics single ionization O2 strong laser fields wavelength- and polarization-dependence
摘要
实验上,在线偏振和圆偏振强激光场中测得同核双原子分子O2在两个不同波长(800 nm和1500 nm)下的离子产量随光强变化曲线,发现其呈现出有趣的波长和偏振依赖关系: O2+产量在长波长下比短波长下更低,且不同波长间 O2+产量的差距在圆偏振光下相较线偏振下变得更大。利用散射矩阵(S-Matrix)理论模型定性地重复出实验结果,并从电子动量分布方面进一步确认了分子轨道效应对O2强场单电离的影响。
Abstract
In this study, the ion yields of homonuclear diatomic molecules (O2) were experimentally measured as a function of the laser intensity at two different wavelengths (800 and 1500 nm) in the linearly polarized (LP) and circularly polarized (CP) strong laser fields, exhibiting a peculiar dependence on wavelength and polarization. The yields were reduced at long wavelengths, and the yield difference between 800 and 1500 nm was larger in the CP field when compared with that in the LP field. The experimental results were qualitatively reproduced using the S-matrix model. Furthermore, the calculated electron-momentum distributions confirm the effect of the molecular orbitals on the strong-field single ionization of O2.
林志阳, 林宝卿, 蒲继雄. 波长和偏振依赖的O2分子强激光场单电离[J]. 光学学报, 2020, 40(8): 0802001. Zhiyang Lin, Baoqing Lin, Jixiong Pu. Wavelength- and Polarization-Dependent Single Ionization of O2 in Strong Laser Fields[J]. Acta Optica Sinica, 2020, 40(8): 0802001.