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Facile preparation of silver nanoparticles in bulk silicate glass by high-repetition-rate picosecond laser pulses

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Abstract

One-step precipitation of Ag nanoparticles in Ag+-doped silicate glasses was achieved through a focused picosecond laser with a high repetition rate. Absorption spectra and transmission electron microscopy (TEM) confirmed that metallic Ag nanoparticles were precipitated within glass samples in the laser-written domain. The surface plasmon absorbance fits well with the experimental absorption spectrum. The nonlinear absorption coefficient β is determined to be 2.47 × 10-14 m/W by fitting the open aperture Z-scan curve, which originated from the intraband transition in the s-p Ag band. The formation mechanism of Ag-glass nanocomposites is discussed as well.

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DOI:10.3788/COL202119.011901

所属栏目:Nonlinear Optics

基金项目:This work was supported by the National Key Research and Development Program of China (No. 2016YFB1102405), National Natural Science Foundation of China (No. 61675214), and Shanghai Sailing Program (No. 20YF1455200).

收稿日期:2020-06-28

录用日期:2020-09-04

网络出版日期:2020-12-02

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沈丹阳:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China;Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
钱 静:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China;Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
王承伟:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China;Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
王关德:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China;Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
王雪辉:Technology Center, Huagong Laser Engineering Co., Ltd., Wuhan 430000, China
赵全忠:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China;Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

联系人作者:赵全忠(zqz@siom.ac.cn)

备注:This work was supported by the National Key Research and Development Program of China (No. 2016YFB1102405), National Natural Science Foundation of China (No. 61675214), and Shanghai Sailing Program (No. 20YF1455200).

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引用该论文

Danyang Shen, Jing Qian, Chengwei Wang, Guande Wang, Xuehui Wang, Quanzhong Zhao, "Facile preparation of silver nanoparticles in bulk silicate glass by high-repetition-rate picosecond laser pulses," Chinese Optics Letters 19(1), 011901 (2021)

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