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Periphery excitation of laser-induced CN fluorescence in plasma using laser-induced breakdown spectroscopy for carbon detection

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Abstract

Carbon is hard to be sensitively detected in laser-induced breakdown spectroscopy (LIBS). The optical emission can be significantly enhanced by resonantly exciting CN radicals in the plasma center using LIBS assisted with laser-induced fluorescence (LIBS-LIF). However, the nitrogen source for CN formation is provided by ambient gas. Therefore, we propose a new approach of periphery excitation in plasma to improve CN fluorescence. The optical and spatial characteristics of CN radicals in plasma were discussed. A fluorescence map was established by combining focal point location and fluorescent intensity, demonstrating that plasma periphery had 4.2 times stronger fluorescence than the center.

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DOI:10.3788/COL202018.083001

所属栏目:Spectroscopy

基金项目:This work was supported by the National Key Research and Development Program of China (No. 2017YFB-1104500), Key-Area Research and Development Program of Guangdong Province (No. 2020B090922006), Guangdong Basic and Applied Basic Research Foundation (No. 2019A1515111120), Science and Technology Program of Guangzhou (No. 202002030165), Featured Innovation Project of Guangdong Education Department (No. 2019KTSCX034), Young Innovative Talents Project in Universities of Guangdong Province (No. 2018KQN-CX057), and Young Scholar Foundation of South China Normal University (No. 19KJ13).

收稿日期:2020-05-09

录用日期:2020-06-10

网络出版日期:2020-07-09

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赵楠:Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631, China;Guangzhou Key Laboratory for Special Fiber Photonic Devices, South China Normal University, Guangzhou 510631, China
李嘉铭:Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631, China;Guangzhou Key Laboratory for Special Fiber Photonic Devices, South China Normal University, Guangzhou 510631, China;Guangdong Provincial Key Laboratory of Industrial Ultrashort Pulse Laser Technology, Shenzhen 518055, China
马琼雄:Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631, China;Guangzhou Key Laboratory for Special Fiber Photonic Devices, South China Normal University, Guangzhou 510631, China;Guangdong Provincial Key Laboratory of Industrial Ultrashort Pulse Laser Technology, Shenzhen 518055, China
郭亮:Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631, China;Guangzhou Key Laboratory for Special Fiber Photonic Devices, South China Normal University, Guangzhou 510631, China;Guangdong Provincial Key Laboratory of Industrial Ultrashort Pulse Laser Technology, Shenzhen 518055, China
张庆茂:Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631, China;Guangzhou Key Laboratory for Special Fiber Photonic Devices, South China Normal University, Guangzhou 510631, China;Guangdong Provincial Key Laboratory of Industrial Ultrashort Pulse Laser Technology, Shenzhen 518055, China

联系人作者:李嘉铭(jmli@m.scnu.edu.cn)

备注:This work was supported by the National Key Research and Development Program of China (No. 2017YFB-1104500), Key-Area Research and Development Program of Guangdong Province (No. 2020B090922006), Guangdong Basic and Applied Basic Research Foundation (No. 2019A1515111120), Science and Technology Program of Guangzhou (No. 202002030165), Featured Innovation Project of Guangdong Education Department (No. 2019KTSCX034), Young Innovative Talents Project in Universities of Guangdong Province (No. 2018KQN-CX057), and Young Scholar Foundation of South China Normal University (No. 19KJ13).

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引用该论文

Nan Zhao, Jiaming Li, Qiongxiong Ma, Liang Guo, Qingmao Zhang, "Periphery excitation of laser-induced CN fluorescence in plasma using laser-induced breakdown spectroscopy for carbon detection," Chinese Optics Letters 18(8), 083001 (2020)

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