光学 精密工程, 2017, 25 (7): 1777, 网络出版: 2017-10-30  

气溶胶颗粒折射率在光学粒径测量中的影响

Impact of refractive index of aerosol particles on particle diameter optical measurement
左晨泽 1,2,*吕且妮 1,2葛宝臻 1,2
作者单位
1 天津大学 精密仪器与光电子工程学院,天津 300072
2 光电信息技术教育部重点实验室, 天津 300072
摘要
针对单颗粒光散射测量方法中被测颗粒折射率会影响测量结果的问题, 根据Mie理论和光辐射能通量计算公式, 对13种常见气溶胶颗粒, 在不同采光中心角θ和采光接收半角β下的散射光辐射能通量F与粒径D关系曲线进行了计算, 提出一种基于相对测量误差平均值的评价标准, 依据该评价标准定量分析了13种折射率对测量的影响。通过对模拟结果的分析, 得出采光结构接收到的光辐射能通量包含前向散射光的条件下, 13种颗粒的F-D曲线较为接近, 折射率对测量结果的影响相对较小。
Abstract
Regarding the negative effect of refractive index of particles in single particle light scattering measurement, the relationship curves between the scattering radiant flux F and the particle diameter D were calculated for 13 kinds of common aerosol particles at different light-receiving central angle θ and light-receiving half-angle β, according to the Mie theory and the light radiant flux calculation formula. Thereby an evaluation standard based on the average of the measured relative errors was presented and employed to evaluate the impact of 13 kinds of refractive index on the measurement quantitatively. Through the analysis of simulation results, it is concluded that if the light radiant flux received by the light-receiving system includes the forward scattered light, the F-D curves of 13 kinds of particles are close to each other, and the impact of refractive index in the measurement is remarkablely reduced.
参考文献

[1] 韩永, 王体健, 饶瑞中, 等. 大气气溶胶物理光学特性研究进展[J]. 物理学报, 2008, 57(11): 7396-7407.

    HAN Y, WANG T J, RAO R ZH, et al.. Progress in the study of physic-optics characteristics of atmospheric aerosols [J]. Acta Physica Sinica, 2008, 57(11): 7396-7407. (in Chinese)

[2] BARON P A, WILLEKE K. Aerosol Measurement: Principles, Techniques, and Applications [M]. 2nd ed.. New York: John Wiley & Sons, 2005.

[3] LEE S H, ALLEN H C. Analytical measurements of atmospheric urban aerosol [J].Analytical Chemistry, 2012, 84(3): 1196-1201.

[4] KUHLI M, WEISS M, STECKEL H. A new approach to characterise pharmaceutical aerosols: measurement of aerosol from a single dose aqueous inhaler with an optical particle counter [J]. European Journal of Pharmaceutical Sciences, 2010, 39(1-3): 45-52.

[5] YOUTHAPOLNAVEE A, CHEWPRADITKUL W, CHAISAWADI A. A construction of particle counter by using laser light scattering [C]. 6th International Conference on Electrical Engineering/Electronics, Computer, Telecommunications and Information Technology, IEEE, 2009: 452-455.

[6] NAGY A, SZYMANSKI W W, GL P,et al.. Numerical and experimental study of the performance of the dual wavelength optical particle spectrometer (DWOPS) [J]. Journal of Aerosol Science, 2007, 38(4): 467-478.

[7] MILES R E H, CARRUTHERS A E, REID J P. Novel optical techniques for measurements of light extinction, scattering and absorption by single aerosol particles [J].Laser & Photonics Reviews, 2011, 5(4): 534-552.

[8] PINNICK R G, PENDLETON J D, VIDEEN G. Response characteristics of the particle measuring systems active scattering aerosol spectrometer probes [J].Aerosol Science and Technology, 2000, 33(4): 334-352.

[9] SZYMANSKI W W, LIU B Y H. On the sizing accuracy of laser optical particle counters [J].Particle & Particle Systems Characterization, 1986, 3(1): 1-7.

[10] 许德毓, 蔡小舒. 激光散射法测量TSP和PM10的最佳采光角及立体角的研究[J]. 上海理工大学学报, 2001, 23(1): 57-60, 65.

    XU D Y, CAI X SH. A theoretical study on light scattering method for measuring TSP and PM10 [J]. Journal of University of Shanghai for Science and Technology, 2001, 23(1): 57-60, 65. (in Chinese)

[11] 葛宝臻, 钟现奎, 刘俊杰, 等. 基于激光散射法的气溶胶颗粒测量系统的接收参数分析[J]. 天津大学学报: 自然科学与工程技术版, 2013, 46(1): 22-28.

    GE B ZH, ZHONG X K, LIU J J,et al.. Reception parameters of aerosol particle measurement system based on light scattering method [J]. Journal of Tianjin University: Science and Technology, 2013, 46(1): 22-28. (in Chinese)

[12] MIE G. Beitrge zur optik trüber medien, speziell kolloidaler metallsungen [J]. Annalen der Physik, 1908, 330(3): 377-445.

[13] VAN DE HULST H C. Light Scattering by Small Particles [M]. New York: John Wiley & Sons, 1957.

[14] SZYMANSKI W W,NAGY A, CZITROVSZKY A. Optical particle spectrometry-problems and prospects [J]. Journal of Quantitative Spectroscopy and Radiative Transfer, 2009, 110(11): 918-929.

[15] PINNICK R G, PENDLETON J D, VIDEEN G. Response characteristics of the particle measuring systems active scattering aerosol spectrometer probes [J]. Aerosol Science and Technology, 2000, 33(4): 334-352.

[16] PESCHL U. Atmospheric aerosols: composition, transformation, climate and health effects [J]. Angewandte Chemie International Edition, 2005, 44(46): 7520-7540.

[17] WANG H B, SHI G M, TIAN M, et al.. Aerosol optical properties and chemical composition apportionment in Sichuan Basin, China [J]. Science of the Total Environment, 2017, 577: 245-257.

[18] HAN T T, XU W Q, CHEN C,et al.. Chemical apportionment of aerosol optical properties during the Asia-Pacific Economic Cooperation summit in Beijing, China [J]. Journal of Geophysical Research: Atmospheres, 2015, 120(23): 12281-12295.

[19] HAND J L, KREIDENWEIS S M. A new method for retrieving particle refractive index and effective density from aerosol size distribution data [J].Aerosol Science and Technology, 2002, 36(10): 1012-1026.

左晨泽, 吕且妮, 葛宝臻. 气溶胶颗粒折射率在光学粒径测量中的影响[J]. 光学 精密工程, 2017, 25(7): 1777. ZUO Chen-ze, L Qie-ni, GE Bao-zhen. Impact of refractive index of aerosol particles on particle diameter optical measurement[J]. Optics and Precision Engineering, 2017, 25(7): 1777.

关于本站 Cookie 的使用提示

中国光学期刊网使用基于 cookie 的技术来更好地为您提供各项服务,点击此处了解我们的隐私策略。 如您需继续使用本网站,请您授权我们使用本地 cookie 来保存部分信息。
全站搜索
您最值得信赖的光电行业旗舰网络服务平台!