Non-scanning systems for far-infrared radiation detection from laser-induced plasmas Download: 779次
1. General review on THz detectors
Nowadays, detection of radiation in the terahertz (THz) frequency domain is of great interest in active research[1, 2]. Generally speaking, the methods involved can be mainly categorized into two types: incoherent (direct) detection and coherent detection. In order to meet the requirements of different applications, designs for specific THz radiation detection systems need to take the following three factors into account: (1) whether the system has sufficiently high sensitivity to allow signals to be extracted from thermal background radiation; (2) whether the data sampling rate allows real-time measurements of ultrafast processes; and (3) whether full characterization of the THz radiation, including amplitude and phase information, can be provided with no or little distortion. The last requirement cannot be achieved other than by using coherent detectors/methods.
Spectral information is always considered essential in real applications. For applications that require very high spectral resolution within a known frequency region, heterodyne detection systems based on frequency mixing are preferred. At room temperature, a semiconductor-based detector, such as a planar Schottky-diode mixer, is combined with a local oscillator for frequency downconversion[3, 4]. The created downshifted signal – the intermediate-frequency (IF) signal – is then filtered and amplified to obtain high sensitivity of detection, the noise equivalent power (NEP) of which is typically on the order of . Cryogenic-cooling techniques are used in heterodyne systems to provide even smaller NEPs of . The most widely used superconducting heterodyne detector includes the superconductor–insulator–superconductor (SIS) tunnel junction mixer[5]. In principle, the detectable frequency range of a heterodyne system is determined by the operating frequency of the local oscillator, which is normally in the sub-THz or low-THz frequency region. The corresponding response time is on the level of picoseconds.
For broadband detection, direct detectors based on thermal absorption are widely used. Room-temperature thermal-type detectors include pyroelectric detectors and Golay cells. Bolometers can also be operated at room temperatures, though helium-cooling technologies are always provided to reduce background thermal noise. Compared with heterodyne devices, direct detectors have typical response times of milliseconds and suffer from a much higher NEP value (typ. for room temperature; for helium-cooled systems). The responsivity of a thermal-type direct detector usually shows little dependence on radiation wavelength; hence bandpass filters or interferometric measurements are generally involved in providing spectral information of the measured signals. A Fourier transform infrared (FTIR) spectrometer, which is commonly used for the identification and analysis of materials with frequency structures in the THz domain, is operated in conjunction with a far-infrared (FIR) optical interferometer and a direct detector. Moreover, since FIR interferometry is based on the autocorrelation effects of THz pulses, it can also be used to measure the pulse duration of FIR signals[6].
With the rapid development of ultrafast laser systems, pulsed detectors based on photoconductive or free-space electro-optic (EO) sampling are generally used for coherent detection of broadband THz radiation. The detection scheme excludes the majority of background noise from the time measurement window, and the signal–noise ratio (SNR) of detection surpasses 104 using lock-in technologies[7]. Comparing photoconductive- and EO-based detection systems, the spectral response of the former is affected by the carrier lifetime as well as by antenna structures[8], while the latter, as a pure optical technique, is considered more reliable in providing a flat frequency response over a wider frequency domain by using short probe pulses. Detectable frequencies in excess of 20 and 100 THz have been demonstrated using photoconductive-[9] and EO-sampling[10] detectors, respectively. THz time–domain spectroscopy (THz–TDS), which has been developed on the basis of pulsed THz techniques, is now widely used to study material properties and transient processes in the FIR region.
The effective spectral response range of EO detection systems is ultimately determined by[11]: (1) the group-velocity mismatch (GVM) between THz and probe pulses; and (2) the phonon absorption of EO crystals. ZnTe and GaP are two of the most commonly used sensors for EO sampling. The former shows excellent detection sensitivity around 2 THz due to the small GVM of optical/THz pulses within the tuning range of Ti:sapphire lasers[12], while the latter has a high fundamental transverse-optical (TO) phonon resonance frequency near 11 THz[13]. Generally speaking, thinner EO crystals tend to provide a wider spectral response at the cost of detection sensitivity. The effective use of a -cut ZnTe crystal is narrowed by about 40% (from 4 to 2.5 THz) as the crystal thickness is changed from 0.2 to 1 mm[14, 15]. In considering the trade-off between high detection sensitivity and broadband spectral response, the type and thickness of EO crystals should be chosen carefully for specific research.
2. Non-scanning schemes based on EO sampling
One of the main drawbacks of conventional EO-sampling techniques is the low acquisition rate. Normally, the read-out time for a single THz waveform would be at least seconds using serial acquisition schemes, which limits the application of this technique for real-time measurements of fast-moving objects or for real-time imaging. Moreover, how to maintain a high SNR of detection while operating the lock-in amplifier with a low time constant has always been an issue in fast scanning[7].
To increase the data acquisition rate, conventional single-channel delay-scanning detection should be replaced by parallel data collection and multi-channel detector arrays. Much effort has been made in developing ‘single-shot’ (non-scanning) EO detection systems since 1998, and in general the techniques are progressing in two directions: spectral encoding[16] and spatial encoding[17]; see Figures
To achieve both high sensitivity and temporal resolution, a third ‘single-shot’ EO-cased technique has been introduced as a cross-correlation technique by second-harmonic generation (SHG)[19], as depicted in Figure
Based on the schemes (including algorithms) shown in Figures
3. True single-shot THz diagnostics in intense laser–plasma interactions
The development of THz sciences is in great need of high-power THz sources. With the rapid development of ultrashort laser systems, laser–plasma interactions as a new field of research have received considerable attention for strong THz radiation generation[6, 22–26]. However, with increasing laser energies, the repetition rates and stability of laser systems are both decreased. The sensitivity of laser–plasma interactions to small laser fluctuations has motivated the development of true single-shot THz-diagnostic techniques.
3.1. Incoherent detection
Direct measurements based on thermal absorption are still by far the most convenient and widely used methods for the detection of broadband plasma-based THz sources. In order to obtain spectral information in one laser shot, multi-channel detection with bandpass or low-pass filters is preferred, as depicted in Figure
Fig. 3. Schematic of a multi-channel THz-diagnostic system based on a direct detector array.
3.2. Coherent detection
THz pulses generated from ultrafast laser–plasma interactions are often characterized by pump and probe measurements. Traditional pump–probe schemes such as EO sampling, which relies on lock-in techniques, are very sensitive to laser noise (which can be quite substantial at low repetition rates) and low-frequency disturbance. For intense laser–plasma interactions, the low repetition rate and relatively large laser fluctuations have motivated the development of true single-shot EO-based measurements. In principle, the non-scanning schemes introduced in Section
3.2.1. Single-shot interferometric scheme using frequency-domain holography
Spectral interferometry, which is also called Fourier-domain interferometry (FDI), is a well-known linear technique for phase and amplitude retrieval from an unknown field in the femtosecond domain[27]. Normally, multiple shots are required to obtain the complete temporal field, but the acquisition rate can be greatly increased by using linearly chirped probe pulses. The in-line interferometric scheme is considered unsuitable for true single-shot THz field diagnostics, since a reference shot has to be recorded as the background before performing the signal retrieval[20]. We proposed a modified scheme using single-shot frequency-domain holography (FDH)[28], as depicted in Figure
Fig. 4. Spectral interferometry scheme using twin-chirped-pulse FDH (quoted from Ref. [28]).
3.2.2. Single-shot THz-pulse characterization by dual echelon optics
In the 2000s, dual echelon optics was first employed to single-shot THz diagnostics[29]. The main idea is to divide the transverse profile of a probe beam by stair-step (echelon) structures into multiple delayed beamlets, which are then focused onto the same spot on an EO crystal to monitor the phase modulation caused by a copropagating THz pulse. The portions of probe beamlets with THz temporal information encoded on them are sequentially imaged onto different positions of a CCD camera for single-shot image processing. To maximize the number of sampling points within one laser shot, two orthogonally oriented echelons are used (rather than one) to fully subdivide the transverse probe beam profile, which has been pre-magnified in diameter. The so-called echelon optics technique, as depicted in Figure
Fig. 5. Schematic of single-shot THz measurement using dual echelon optics (quoted from Ref. [29]).
3.3. Infrared streak camera
Most electronic devices cannot be used for the direct measurement of fast transient processes in the picosecond region, with the exception of streak cameras. The spectral response of a streak camera is determined by the photocathode material, most of which are sensitive only to electromagnetic radiation of wavelengths shorter than . By using gas-phase Rydberg atoms as the cathode, the measurable wavelength can be extended to the FIR region[30]. Alternatively, by placing an EO crystal as a converter before an optical streak camera, THz pulses can be retrieved indirectly by measuring copropagating long probe pulses[31]. Comparing an atomic streak camera and an EO-based infrared streak camera, the former can provide information only on the time envelope of THz waves, while the latter is in principle a coherent measurement (but requires an additional reference shot for THz field diagnosis). The temporal resolution of infrared streak camera systems is not comparable to that which can be achieved by single-shot EO-based optical systems.
4. Summary and outlook
In this paper, we present an overview on the state-of-the-art techniques for single-shot THz diagnostics involved in intense laser–plasma interactions. For incoherent detection, direct detectors can be used with THz filters to provide general spectral information. Atomic infrared streak cameras, which operate in the infrared regime (typ. from 1 to ), are able to measure the intensity profile of THz pulses directly, with a time resolution of about one picosecond. For coherent detection, a THz field can be retrieved via single-shot EO-sampling techniques, either by time-to-space or time-to-spectrum conversion. Associated with specific applications, THz-diagnostic systems should be carefully designed according to the experimental and laser conditions. Practically speaking, high detection sensitivity is always the first concern, followed by high time resolution. Efforts toward higher-power THz sources and an improved understanding of THz radiation under extreme conditions, would promise continuing advances in single-shot THz technologies for intense laser–plasma interactions.
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[4]
[5]
[6]
[7]
[8]
[9]
[10]
[11]
[12]
[13]
[15]
[16]
[17]
[18]
[19]
[20]
[21]
[22]
[23]
[24]
[26]
[27]
[29]
Article Outline
Chun Li, Guo-Qian Liao, Yu-Tong Li. Non-scanning systems for far-infrared radiation detection from laser-induced plasmas[J]. High Power Laser Science and Engineering, 2015, 3(2): 02000001.