光纤激光器被动锁模技术研究进展 下载: 3143次特邀综述
Signature For the past two decades, ultrafast fiber lasers have become fundamental building blocks in many applications, such as optical communications, biomedical imaging, and industrial processing. Passive mode-locking techniques have been investigated. The nonlinear saturable absorption (SA) effect is the core of the passive mode-locking technology of fiber lasers. Passive mode-locking techniques can be categorized into real and artificial saturable absorbers. The real saturable absorbers consist of semiconductor saturable absorption mirrors (SESAM) and nanomaterials. The artificial saturable absorbers consist of the nonlinear polarization rotation evolution (NPE), nonlinear optical loop mirror (NOLM), nonlinear multimode interference (NLMMI), and Mamyshev regenerator (Mamyshev). The abovementioned passive mode-locking technologies have their advantages and disadvantages. In this study, we briefly illustrate their pros and cons and review their recent development in various types of saturable absorption effects in the application of ultrafast pulse generation.
For real saturable absorbers, rising from the extraordinary physical, optical, and electronic properties of graphene in 2004, layered-dependent nanomaterials have attracted significant attention because of their advantages of cost-effectiveness, broadband optical response, high nonlinear, fast relaxation, and flexible compatibility with other photonics structures. The optical modulation effect of nanomaterials provides a pulse shaping mechanism (i.e., reduced absorption with increasing optical intensity); thus, it can support stable pulse generation and operation in a laser system. Most optical modulators are based on the third-order nonlinear optical response of nanomaterials, such as saturable absorption and optical Kerr effects. SA is a process originating from valance band depletion, conduction band filling, and ultrafast intra-band carrier relaxation exhibited by the input power-dependent optical absorption. Various nanomaterial-based SAs have been demonstrated for pulse generation in fiber lasers operating from the visible to mid-infrared regions. For the artificial saturable absorbers, these passive mode-locking technologies including NPE, NOLM, NLMMI, and Mamyshev could generate ultrashort, high repetition ratio, and high peak power pulses with demand. The optical modulation effect of artificial saturable absorbers originates from the operating optical properties: NPE technique using the optical properties of polarization, NOLM technique using optical nonlinear interference, NLMMI technique utilizing nonlinear multimode interference, and Mamyshev mode-locking technique using nonlinear self-phase modulation. These artificial SAs could largely tune optical modulation depths and enable some types of pulse generation.
The above-mentioned passive mode-locking techniques have progressed considerably. NOLM mode-locking fiber laser has been used in frequency comb applications due to its high repetition ratio feature. Mamyshev mode-locking fiber laser-generated ultra-high peak power pulses could be compared to commercial Ti: Sapphire lasers. NPE mode-locking fiber lasers could largely tune operating pulse states, acting as an ideal seed source for laser amplifier systems. Mode-locking fiber lasers made of nanomaterials have wide application prospects due to their flexible features. With increasing demand for fiber lasers, the above-mentioned traditional passive mode-locking techniques need to improve their performances. Thus, we review the recent advancement of these techniques to illustrate how they overcome their disadvantages.
Progress There are two solutions to improve the stability of the NPE passive mode-locking technique. The first one is to replace traditional fiber with polarization maintaining (PM) fiber (
Conclusions and Prospects As the mechanism of saturable absorber effects for mode-locked fiber lasers are clear, researchers will be able to choose appropriate mode-locking mechanisms to satisfy the specific demands of end-users. Finally, the recent progress of ultrafast fiber lasers poses a new challenge; thus, more investigation is required.
1 引言
超快光纤激光在**、科研、工业以及医疗等领域均具有重要应用[1]。光纤激光器具有光束质量好、热管理效率高、结构灵活紧凑和维护成本低等优势[2]。光纤作为柔性波导,在赋予光纤激光器以上所述优势的同时,也引入了色散和非线性效应[3]。脉冲在光纤中传输时,较小的纤芯波导容易产生较高的功率密度,所激发的非线性效应会累积较高的非线性相移导致脉冲分裂为多个脉冲或者塌陷为类噪声脉冲,这极大地限制了超快光纤激光输出的脉冲能量与峰值功率。为了产生超快光纤激光,平衡或者抑制非线性效应成为关键。其中一种有效方案为增加模场面积,抑制非线性响应。因此,拥有较大模场面积的光子晶体光纤技术得到飞速发展。另一种方案是通过控制谐振腔内的色散来平衡非线性效应。在负色散域,由于色散和非线性平衡而形成的脉冲称为孤子,其峰值功率受限于孤子面积理论[4]。为了打破负色散对脉冲功率的限制,采用色散管理脉冲即腔内包含正色散和负色散两部分光纤,在正色散域拉伸脉冲降低峰值功率,在负色散域压缩脉冲提升峰值功率并输出,可使脉冲输出功率提升一个数量级[5]。色散管理孤子依然受到腔平均色散孤子面积理论的约束,致使其功率无法进一步提升。去除负色散光纤使光纤激光器工作在全正色散域,同时腔内引入滤波器增加频域损耗可以获得耗散孤子[6-7]。脉冲能量的典型值为20 nJ,脉冲宽度约为200 fs,进一步提升了峰值功率。另外,自相似子也是获得大能量的方式之一,其特点是脉冲在腔内传输过程中维持抛物线形状并且始终为线性啁啾[8-9]。为了控制腔内自相似运转,采用两种方式,一种是被动自相似子的方式即从时域控制,在输出位置之后引入色散延迟器件;另一种是放大自相似子的方式即从频域控制,在增益放大之后引入窄带滤波器件。这些方式都能在一定程度上提升脉冲能量,但是依然受限于非线性相移和连续光干扰等因素影响无法进一步提升脉冲峰值功率。
为了进一步提升超快光纤激光的输出性能以满足光频率梳、太赫兹、生物光子学等应用的需求,对于锁模光纤激光器来说,深入理解并合理利用非线性效应成为关键所在。从被动锁模光纤激光器产生锁模脉冲的机理来看,波导介质引起的群速度色散、非线性效应,滤波器的频谱滤波效应,以及可饱和吸收体(SA)引起的自振幅调制效应等物理过程之间的相互平衡是形成稳定脉冲的关键因素[10],本文将重点论述基于可饱和吸收效应被动锁模技术的研究进展。可饱和吸收体是利用非线性效应产生超快光纤激光的被动光调制器件,其光调制作用一般是指衰减光强的能力随光强的增大而降低[11]。可饱和吸收体的实现方式分为真实饱和吸收体和人造饱和吸收体。真实饱和吸收体包括半导体可饱和吸收镜(SESAM)[12]和纳米材料[13];人造可饱和吸收体包括非线性多模干涉(NLMMI)[14]、非线性偏振演化(NPE)[15]、非线性光环形镜(NOLM)[16]和Mamyshev再生器(Mamyshev)[17],可饱和吸收体的不同实现方式如
合理选择可饱和吸收体参数是获得具有自启动、高环境稳定性、脉冲参数可控等特点的超快光纤激光的核心技术。在被动锁模技术应用中,各种可饱和吸收体被动锁模技术产生超短光纤激光的优势以及所面临的问题不同。NPE锁模技术具有波长可调、调制深度大、响应时间短等优点,但是工作状态会受到环境温度、外部振动、偏振退却等因素的影响,使NPE等效的可饱和吸收体参数在长时间工作条件下易发生变化导致锁模状态发生变化甚至失锁[22];NOLM锁模技术具有环境稳定性高、响应时间短等特点,但是等效的可饱和吸收体调制深度主要受到耦合比的影响。较小的耦合比需要更长的光纤来累积非线性相移而无法获得高重复频率、窄脉冲,更容易得到耗散孤子共振(DSR)或者类噪声(NLP)等[23],较大的分光比可以在较短的光纤内累积足够的非线性相移产生超快光纤激光但是难以自启动;Mamyshev振荡器锁模技术可以提供较大的调制深度,获得高峰值功率的超短脉冲且可以充分地抑制连续光分量等造成的脉冲不稳定,缺点是无法从噪声中自起振[24];SESAM工艺成熟、稳定性较高,缺点是无法实现宽带响应、响应时间较长、特殊结构无法实现全光纤结构设计[25];Nano-materials可饱和吸收体优点是成本较低、易于集成、宽带响应,缺点是热损伤阈值较低、长时间工作稳定性有待提升[19];NLMMI优点是全光纤结构、制备成本低,缺点是特殊结构会增大腔损耗,可饱和吸收体参数的可调性、环境稳定性较差[14]。以上所述各类可饱和吸收体的实现方式所面临的问题都亟须解决。因此,本文总结了最近各类等效可饱和吸收体被动锁模光纤激光器的发展方向,同时简要阐明工作原理、技术优势、解决问题的方法以及应用领域。
2 非线性偏振演化锁模技术
非线性偏振旋转演化锁模技术是克尔效应引起的不同偏振光产生不同非线性相移而实现可饱和吸收效应的锁模机制。NPE形成的等效可饱和吸收体可以用
如何规避或者抵消NPE锁模环境不稳定性的缺点?近几年,全保偏光纤NPE锁模和智能NPE锁模逐渐成为解决NPE技术问题的两个主要方向。全保偏NPE锁模的核心技术是将标准单模光纤替换为保偏光纤,可以规避掉单模光纤弱双折射效应引起的调制不稳定性,进而提升激光腔的整体环境稳定性;智能NPE锁模的核心技术是通过智能算法与控制系统相结合的方式,自动反馈并自动调控激光腔内的偏振状态。当腔内偏振状态由于外部环境发生变化时,智能系统可以迅速甄别并自动调节偏振器件,进而抵消掉NPE光纤激光器对环境的敏感性。
对于全保偏NPE锁模光纤激光器来说,保偏光纤中光场的偏振态受外界影响较小,在传播过程中状态不易改变。保偏光纤的拍长非常短约为2 mm,两正交偏振光会在保偏光纤中传输时发生走离从而减弱非线性调制效应,因此对于全保偏NPE锁模技术走离效应的补偿尤为重要。2017年,Szczepanek等[29]利用多段保偏光纤角度熔接补偿走离效应,实现了全保偏光纤NPE锁模,实验装置如
图 3. 全保偏光纤NPE锁模激光器实验装置图以及可饱和吸收效应原理图[24]
Fig. 3. All-polarization-maintaining fiber NPE mode-locking fiber laser setup and the mechanism of saturable absorption effect[24]
对于智能锁模NPE来说,它可以克服NPE锁模激光器环境敏感性的缺点和提升NPE锁模技术的主动控制能力。智能锁模的开端是利用外部电压控制液晶可变器,建立外部电压与锁模状态的关系,从而达到通过调控外部电压值来调控激光器运转状态的目的[31]。随后,利用演化算法(EA)的自组织、自适应、自学习特点,只需以几个实验参数为最初的“父代”,EA算法就可以自己通过“子代”迭代的方式来寻找目标结果,即锁模状态[32]。为了提升智能锁模的智能性,深度学习(DL)和模型预测控制(MPC)算法可以自己识别锁模脉冲域并建立物理模型定义这些脉冲域,并可以自行调节参数重现这些不同的锁模脉冲域[33]。为了提升智能锁模的响应调控速率,类人算法(HLA)的优势在于对目标锁模状态设置目标函数,可快速识别目标域,从而极大地提升了智能锁模的调控速率[34]。
智能锁模利用时间拉伸色散傅里叶变换(TSDFT)作为光谱判别的快速分析技术,并采用智能偏振选择算法相结合的方式。其特点是可快速响应并调控各脉冲域,并且还可以直接观测到各脉冲域之间切换的过渡态[35]。智能锁模光纤激光器的实验装置如
图 4. 智能NPE锁模光纤激光器实验装置[30]
Fig. 4. Experimental setup of intelligence NPE mode-locking fiber laser[30]
3 非线性光环形镜锁模技术
利用Sagnac环产生强度相关的非线性相移差实现锁模的激光器称为NOLM锁模激光器,类似于数字“8”,也称为8字型腔激光器[37]。形成的可饱和吸收效应可以用
为了提高8字腔光纤激光器的环境稳定性,全保偏8字腔锁模光纤激光器成为热点研究方向。全保偏8字腔提升环境稳定性的核心技术同全保偏NPE锁模技术类似,都是将标准单模光纤替换为保偏光纤,提升激光腔的环境稳定性。不同之处在于,8字腔结构不存在群速度失配的问题,腔型设计相对简单。典型的全保偏8字腔结构如
图 6. 全保偏8字型锁模光纤激光器实验装置图[32]
Fig. 6. Experimental setup of all-polarization-maintaining figure 8 mode-locking fiber laser[32]
为了满足高重复频率如光频梳等应用,获得高重复频率激光输出的最直接的技术方案为缩短激光腔长,但对于NOLM激光器来说,短腔无法保证积累足够的非线性相移。2016年 Jiang等[43]将反射式相位偏置器置入到9字腔腔内实现自启动。相位偏置器是由分束器、FR、1/8波片和反射镜组成,主要作用是使光场延迟π/2,可饱和吸收体的透过率曲线发生平移,并手动调谐到适合建立锁模的区域。全光纤结构下输出脉冲的最高重复频率可达159 MHz。为了进一步提升重复频率,2018年Liu等[44]通过引入空间器件,在9字腔内引入FR实现了700 MHz的高重复频率脉冲输出,如
图 7. 高重复频率9字腔锁模光纤激光器实验装置图[34]
Fig. 7. Experimental setup of high-repetition figure 9 mode-locking fiber laser[34]
与其他锁模机制相比,NOLM锁模技术对波长不敏感,腔损耗可容忍度较大。为了提高波长覆盖范围,氟化物玻璃(ZBLAN)光纤8字腔锁模光纤激光器成为热门研究方向[45]。现阶段,可见光波段(380~760 nm)超快激光的产生方式主要是钛宝石激光器、光参量放大系统、近红外波段的倍频等[46]。与近红外波段(1 μm、1.5 μm、2 μm等波段)锁模光纤激光器相比,这些方式的不足之处在于成本过高、封装体积过大、光路较复杂等。可见光波段锁模光纤激光器的发展滞后于近红外波段的主要原因在于:1)传统的稀土离子在可见光波段的增益相对较小,而在可见光波段增益较大的ZBLAN光纤的熔点与硅基光纤的熔点相差较大,熔接较困难且损耗较大[47];2)可见光波段器件包括波分复用器、隔离器、高能量泵浦等制备不够成熟[48-49];3)可见光波段的色散值相对近红外波段更大,对于模式锁定会更加困难[50];4)缺少可见光波段的饱和吸收体[51]。以上都是限制可见光波段超快光纤激光器产生的因素。可见光波段锁模光纤激光器的发展依赖于高增益、低损耗的ZBLAN光纤的制备,同样也依赖于高能量蓝光半导体激光器作为激励源[52]。另外,可见光波段的光纤器件的成熟、宽带响应的材料类饱和吸收体的快速发展,也为可见光波段锁模光纤激光器的发展提供了动力[53-54]。由于二维纳米材料的宽带响应特性,可利用其作为可饱和吸收体在可见光波段光纤激光器中产生调Q脉冲输出[55-56]。虽然光纤激光器相比于固体激光器损耗容忍度更大,但是要获得锁模脉冲输出,需要在已获得调Q输出的基础上进一步优化腔型,减少激光的线性损耗,增强饱和吸收特性[57]。
图 8. 可见光波段NOLM锁模光纤激光器实验装置图[58]。(a)原理图;(b) 635 nm全光线结构8字型DSR光纤激光器照片
Fig. 8. Experimental setup of the visible-wavelength NOLM mode-locked fiber laser[58]. (a) Schematic; (b) photograph of 635 nm all-beam structure figure 8 DSR fiber laser
4 纳米材料类饱和吸收体锁模技术
纳米材料类可饱和吸收体由于其工作波段宽、制备简单、成本低、易集成、恢复时间快等优点,得到了研究人员的广泛关注,因而超快激光也得到了迅速发展[59]。纳米材料对光的吸收率随入射光强的增加而减少时材料具有可饱和吸收特性,其工作原理如
图 9. 纳米材料类可饱和吸收效应原理图[13]
Fig. 9. Schematic diagram of saturable absorption effect of nanomaterials[13]
近几十年,SESAM得到了迅速的发展并实现了商业化。SESAM主要由半导体可饱和吸收体和布拉格反射镜组成,以InGaAs量子阱作为可饱和吸收体可以对指定波长实现有效吸收,而在衬底层上交替镀制的GaAs和AlAs层构成的布拉格反射镜决定了反射光谱。Loh等首次提出将SESAM应用于被动锁模光纤激光器。其具有易于自启动、结构简单、性能稳定、锁模阈值低、响应时间短等优点。但其制造工艺复杂、成本较高以及不易于光纤集成等特点促使人们开始寻找其他新型可饱和吸收体。近几年,碳纳米管[61]、石墨烯[62]、拓扑绝缘体[63]、过渡金属硫化物[64]、黑磷[65-66]、MXene[67]和钙钛矿[68]等新型材料相继应用于被动锁模光纤激光器,总结如
纳米材料光器件的光学特性与纳米材料的本质特性如带隙结构、非线性响应系数、载流子浓度、响应恢复时间等直接相关。二维纳米材料与光、电相互作用的机理发展为研制具有光电调控特性的光纤激光器带来了新的发展。2015年,Lee等[78]首次制备了电控全光纤石墨烯器件,通过电场调控该器件,获得激光的调Q和锁模输出。该器件的制备过程是将石墨烯晶体场效应管浸入锂离子液体电解质中,并建立在边抛光纤之上,如
图 11. 电控全光纤石墨烯器件的示意图和图片[78]
Fig. 11. Schematic and image of gate-controlled all-fiber graphene devices[78]
5 非线性多模干涉锁模技术
基模从单模光纤耦合入多模光纤时会激发出高阶模式,高阶模式从多模光纤耦合回单模光纤后会产生非线性模式损耗。研究人员发现这种非线性多模干涉效应可以充当可饱和吸收体,并具有稳定可控、易于使用和集成、适当的饱和通量、超快非线性响应等特点。非线性多模光纤可饱和吸收体的原理如
图 13. SMF-SIMF-GIMF-SMF非线性多模干涉掺Tm光纤激光器[80]
Fig. 13. SMF-SIMF-GIMF-SMF nonlinear multimode interference Tm-doped fiber laser[80]
2019年,Wang等[82]利用一段无芯渐变多模(NCF-GIMF)光纤实现了耗散孤子和束缚态孤子脉冲输出,其光路结构如
图 14. NCF-GIMF非线性多模干涉光纤激光器[82]
Fig. 14. NCF-GIMF NLMMI nonlinear multimode interference fiber laser[82]
6 Mamyshev锁模技术
为了进一步提升光纤激光器的峰值功率,一种新型光纤振荡器即Mamyshev被提出[17]。Mamyshev光纤振荡器包含两个再生放大,每个再生放大都有增益光纤、输出耦合器和滤波器。两个再生放大滤波器的中心波长不同是形成腔内饱和吸收效应、获得大能量高峰值功率的关键[83]。Mamyshev再生放大最早于1998年由Mamyshev提出,随后被应用在通信领域。Mamyshev可饱和吸收体的原理可以用
图 15. Mamyshev再生器可饱和吸收效应原理图[3]
Fig. 15. Schematic diagram of Mamyshev regenerator saturable absorption effect[3]
Mamyshev可饱和吸收体的调制深度为100%,因此可以抑制噪声、连续光成分破坏脉冲输出,缺点是不能够自启动[17],需要注入初始的脉冲信号,这是由于低峰值激光无法保证足够的非线性效应展宽光谱。尽管如此,Mamyshev振荡器在产生高峰值功率上的巨大潜力吸引了研究人员的注意。为了解决Mamyshev振荡器的自启动问题,使用电子可调旋转镜作为脉冲触发装置,
图 17. 理论结果说明190 nJ 脉冲输出[24]。(a)腔内脉冲的光谱演化;(b)脉冲宽度演化(圆圈)和均方根带宽(方块)
Fig. 17. Numerical simulation results for 190 nJ output pulse[24]. (a) Spectral evolution of the pulse in the cavity; (b) evolution of the pulse duration (circles) and RMS bandwidth (squares)
7 结束语
本文梳理了近期利用各类可饱和吸收效应实现锁模的超快光纤激光器研究进展,包括利用偏振损耗锁模的NPR;利用干涉损耗实现锁模的NOLM;利用强度损耗实现锁模的Nanomaterials;利用模式损耗实现锁模的NLMMI;利用SPM非线性频谱损耗实现锁模的Mamyshev。这些锁模机制充分利用了光的偏振、干涉、模式、幅值、非线性等物理特性,为超快锁模光纤激光器在更多的应用场景中应用提供了可能。
超快光纤激光具有重要的应用价值,研究人员期望超快光纤光源更加的稳定、便宜、便携,智能满足日益增加的使用场景。因此熟悉以上所综述的各种非线性可饱和吸收效应锁模机理,设计出满足不同应用需求的超快光纤激光,将有助于推动超快光纤激光器向着更加成熟的方向发展。
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