Controlling multiphoton excited energy transfer from Tm3+ to Yb3+ ions by a phase-shaped femtosecond laser field

Ye Zheng; Lianzhong Deng; Jianping Li; Tianqing Jia; Jianrong Qiu; Zhenrong Sun; Shian Zhang

doi:doi:10.1364/PRJ.7.000486

Photonics Research, 2019, 7 (4): 04000486, Published Online: Apr. 11, 2019

Controlling multiphoton excited energy transfer from Tm3+ to Yb3+ ions by a phase-shaped femtosecond laser field

Ye Zheng ¹Lianzhong Deng ¹Jianping Li ¹Tianqing Jia ¹Jianrong Qiu ²Zhenrong Sun ¹Shian Zhang ^1,3,*

Author Affiliations

¹ State Key Laboratory of Precision Spectroscopy, School of Physics and Materials Science, East China Normal University, Shanghai 200062, China

² State Key Laboratory of Silicon Materials, Zhejiang University, Hangzhou 310027, China

³ Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China

Figures & Tables

Fig. 1. Schematic of the experimental setup. G1 and G2 are two diffraction gratings of 1200 lines/mm each. C1 and C2 are two cylindrical concave mirrors each of focus length 200 mm. SLM, spatial light modulator; λ/4, quarter-wave plate; L1, focusing lens; GA, genetic algorithm.

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Fig. 2. Characterization of the Tm3+/Yb3+ co-doped glass ceramic sample. (a) XRD pattern. (b), (c) TEM images.

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Fig. 3. (a) Absorption spectrum of the Tm3+/Yb3+ co-doped glass ceramics in the UV–VIS–NIR region and (b) the luminescence spectrum of the same sample with the excitation of an 800 nm femtosecond laser pulse.

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Fig. 4. Laser peak intensity dependences of (a) luminescence intensities at 355, 454, 473, and 975 nm for the Tm3+/Yb3+ co-doped glass ceramics and (b) luminescence intensity at 975 nm for the Yb3+ single-doped glass ceramics, together with the absorption (lower right) and luminescence (upper left) spectra.

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Fig. 5. Energy level structures of Tm3+ and Yb3+ ions, together with the proposed mechanisms for explaining the luminescence processes and the energy transfer from Tm3+ to Yb3+ ions.

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Fig. 6. Dependences of luminescence intensities on the value of θ, the angle between the direction of input laser polarization and the optical axis of the λ/4 plate. (a) Luminescence signals at 454 nm (red squares) and 975 nm (blue circles) for the Tm3+/Yb3+ co-doped glass ceramics. (b) Luminescence signal at 975 nm (rose squares) for the Yb3+ single-doped glass ceramics.

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Fig. 7. Optimization processes for (a-1) enhancing and (a-2) suppressing the luminescence signal at 975 nm. Luminescence spectra of the Tm3+/Yb3+ sample with (blue curve) and without (red curve) phase optimization for (b-1) optimal enhancement and (b-2) suppression. Phase masks (blue curve) and laser spectra (red curve) for (c-1) optimal enhancement and (c-2) suppression. Time profiles of the shaped (blue curve) and TL (red curve) femtosecond pulses for (d-1) optimal enhancement and (d-2) suppression.

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Ye Zheng, Lianzhong Deng, Jianping Li, Tianqing Jia, Jianrong Qiu, Zhenrong Sun, Shian Zhang. Controlling multiphoton excited energy transfer from Tm3+ to Yb3+ ions by a phase-shaped femtosecond laser field[J]. Photonics Research, 2019, 7(4): 04000486.

Controlling multiphoton excited energy transfer from Tm3+ to Yb3+ ions by a phase-shaped femtosecond laser field

Fig. 1. Schematic of the experimental setup. G1 and G2 are two diffraction gratings of 1200 lines/mm each. C1 and C2 are two cylindrical concave mirrors each of focus length 200 mm. SLM, spatial light modulator; λ/4, quarter-wave plate; L1, focusing lens; GA, genetic algorithm.

Fig. 2. Characterization of the Tm3+/Yb3+ co-doped glass ceramic sample. (a) XRD pattern. (b), (c) TEM images.

Fig. 3. (a) Absorption spectrum of the Tm3+/Yb3+ co-doped glass ceramics in the UV–VIS–NIR region and (b) the luminescence spectrum of the same sample with the excitation of an 800 nm femtosecond laser pulse.

Fig. 5. Energy level structures of Tm3+ and Yb3+ ions, together with the proposed mechanisms for explaining the luminescence processes and the energy transfer from Tm3+ to Yb3+ ions.

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Controlling multiphoton excited energy transfer from Tm3+ to Yb3+ ions by a phase-shaped femtosecond laser field

Fig. 1. Schematic of the experimental setup. G1 and G2 are two diffraction gratings of 1200 lines/mm each. C1 and C2 are two cylindrical concave mirrors each of focus length 200 mm. SLM, spatial light modulator; λ/4, quarter-wave plate; L1, focusing lens; GA, genetic algorithm.

Fig. 2. Characterization of the Tm3+/Yb3+ co-doped glass ceramic sample. (a) XRD pattern. (b), (c) TEM images.

Fig. 3. (a) Absorption spectrum of the Tm3+/Yb3+ co-doped glass ceramics in the UV–VIS–NIR region and (b) the luminescence spectrum of the same sample with the excitation of an 800 nm femtosecond laser pulse.

Fig. 5. Energy level structures of Tm3+ and Yb3+ ions, together with the proposed mechanisms for explaining the luminescence processes and the energy transfer from Tm3+ to Yb3+ ions.

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